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Jessica Hynes as Mafalda Hopkirk
Chris Miller as Humphries / Magic Mirror (voice)
Laurie Metcalf as Mrs. Davis (voice)
Bobby Block as Baby Bear (voice)
Paul Bettany as Jarvis
Bob Peterson as Additional Voice (voice)
Marcia Wallace as Edna Krabappel
Takayuki Sugou as Shiryu
Bill Hunter as Dentist
Raymond S. Persi as Flash
Estelle Harris as Mrs. Potato Head
Alex Borstein as Barbara Pewterschmidt
Stefan Kapičić as Colossus
Greg Burson as Mr. D.N.A. (voice)
Teddy Newton as Lawyer (Talon Labarthe) (voice)
Teddy Newton as Additional Voices (voice)
Tom Hanks as Woody Car (voice)
Juan Pacheco as Additional voices (voice)
Sam Richardson as Lee the Office Nerd
Bud Luckey as Chuckles (voice)
Ryotaro Okiayu as Kizaru Borsalino
Dan Fogler as Zeng (voice)
Kristen Bell as Priscilla
Helen Mirren as Narrator

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